One-dimensional quantum magnets hosting correlated π-spins and collective quantum behaviour are synthesized through a combination of elegant precursor design and on-surface synthesis, highlighting the potential of designing π-electron-based quantum spin systems for future quantum technologies.
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References
Giamarchi, T. Quantum Physics in One Dimension Vol. 121 (Clarendon Press, 2003).
Anderson, P. W. Mater. Res. Bull. 8, 153–160 (1973).
Lieb, E., Schultz, T. & Mattis, D. Ann. Phys. 16, 407–466 (1961).
Mourigal, M. et al. Nat. Phys. 9, 435–441 (2013).
Mishra, S. et al. Nature 598, 287–292 (2021).
Zhao, Y. et al. Nat. Chem. 15, 53–60 (2023).
Zhao, C. et al. Nat. Nanotechnol. 19, 1789–1795 (2024).
Song, S. et al. Nature 637, 580–586 (2025).
Fu, X. et al. Nat. Synth. https://doi.org/10.1038/s44160-025-00743-5 (2025).
Su, X. et al. Nat. Synth. https://doi.org/10.1038/s44160-025-00744-4 (2025).
Zhao, C. et al. Preprint at https://arxiv.org/html/2408.10045v1 (2024).
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Peng, X., Lu, J. Spin-1/2 Heisenberg chains realized in π-electron systems. Nat. Synth 4, 668–670 (2025). https://doi.org/10.1038/s44160-025-00757-z
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DOI: https://doi.org/10.1038/s44160-025-00757-z
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