The dynamic behavior of supramolecular polymers in aqueous environments remains poorly understood due to the assembly pathway complexity. Here, the authors present a combinatorial titration methodology to probe in situ a binary assembly mechanism between spheroidal micelles and β-sheet polymers of peptide amphiphiles, which collectively govern supramolecular dynamics.
- Huachuan Du
- Ruomeng Qiu
- Samuel I. Stupp
