Abstract
Antiferromagnets have gained a growing interest for next-generation spintronic applications. Among them, the antiferromagnetic Weyl semimetal Mn3Sn stands out because of its electrical and magnetic properties driven by its non-collinear spin structure at room temperature. Despite research progress on the current-induced switching of the magnetic octupole in Mn3Sn, the ultrafast switching inherent to the antiferromagnet remains to be resolved, and the underlying mechanism is yet elusive. Here we measure the spatiotemporally resolved current-induced switching dynamics in polycrystalline Mn3Sn films using ultrafast magneto-optical Kerr effect imaging, with current pulses as short as 140 ps. Our results directly reveal two distinct switching regimes depending on the intensity and duration of the current pulse: a non-thermal process that does not require the transient melting of antiferromagnetic order, and a temperature-assisted process that relies on heating above the magnetic ordering temperature. Our work highlights the potential of Mn3Sn towards ultrafast magnetic recording devices.
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Data that support the findings of this work are available in the Supplementary Information. Source data are provided with this paper.
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Acknowledgements
This work was supported by a JST-MIRAI program (JPMJMI20A1). K.O. acknowledges financial support from JSPS KAKENHI (grant number JP24KJ0653). We are grateful to K. Kondo for fruitful discussions.
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K.O. carried out the optical experiments and analysed the data. K.O. and N.Y. developed the ultrafast TR-MOKE measurement system under the supervision of R.S. H.T. and T. Matsuda optimized the device structure for the TR-MOKE measurements with feedback from K.O., S.N. and R.S. T. Matsuo, Y.T., M.A., H.P. and T.H. grew and characterized the thin films. H.T. fabricated the Hall-bar devices and conducted the transport measurements of current-induced switching phenomena under the supervision of S.N. S.N. and R.S. conceived the project of this study. K.O. and R.S. wrote the manuscript with feedback from all co-authors.
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Ogawa, K., Tsai, H., Yoshikawa, N. et al. Ultrafast time-resolved observation of non-thermal current-induced switching in an antiferromagnetic Weyl semimetal. Nat. Mater. (2025). https://doi.org/10.1038/s41563-025-02402-8
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DOI: https://doi.org/10.1038/s41563-025-02402-8
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