We added lithium (trifluoromethane sulfonyl) imide (LiTFSI) salt into an immiscible poly(methyl methacrylate) (PMMA)/ethylene-vinyl alcohol copolymer (EVOH) to improve the transparency and tensile properties. The addition of LiTFSI reduced the refractive index of EVOH, which matched the refractive index of PMMA, resulting in high transparency. In addition, LiTFSI interrupted the intra- and intermolecular hydrogen bonds between the OH groups in EVOH, resulting in decreased crystallinity. Consequently, the amorphous and flexible EVOH domains in the PMMA matrix changed the tensile properties from brittle to ductile by suppressing the stress concentration.
- Hana Watanabe
- Mayu Horada
- Shogo Nobukawa