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Planckian scattering and parallel conduction channels in an iron chalcogenide superconductor

Abstract

The linear-in-temperature resistivity of cuprate superconductors, which extends in some samples from the superconducting critical temperature to the melting temperature, remains unexplained. Although seemingly simple, this temperature dependence is incompatible with the conventional theory of metals, which dictates that the scattering rate should be quadratic in temperature if electron–electron scattering dominates. Understanding the origin of this temperature dependence and its connection to superconductivity may provide crucial information that helps to understand the superconducting mechanism. Here we show the presence of two conduction channels in the normal state of the iron-based superconductor FeTe1−xSex that add in parallel. One is the broad one in frequency with weak temperature dependence, whereas the other is sharper and has a scattering rate that goes as the Planckian-limited rate that is linear in temperature. This behaviour occurs in two samples, one with almost equal amounts of Se and Te that is believed to be a topological superconductor and the other that is more overdoped. By analysing the spectral weight of the superconducting condensate using our time-domain terahertz spectroscopy measurements, we show that it is mainly drawn from the channel that undergoes Planckian scattering.

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Fig. 1: THz conductivity of the x = 0.45 and x = 0.35 samples.
The alternative text for this image may have been generated using AI.
Fig. 2: Fits to the THz conductivity of the x = 0.45 sample at various temperatures.
The alternative text for this image may have been generated using AI.
Fig. 3: Fit parameters along with d.c. resistivity.
The alternative text for this image may have been generated using AI.
Fig. 4: Superfluid density, three ways.
The alternative text for this image may have been generated using AI.

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Data availability

The data that support the findings of this study are available via Zenodo at https://doi.org/10.5281/zenodo.18662533 (ref. 32). Source data are provided with this paper.

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Acknowledgements

We acknowledge support from the Army Research Office MURI program (W911NF2020166). R.R.III and N.P.A. also acknowledge support from the Gordon and Betty Moore Foundation EPiQS Initiative Grant GBMF-9454.

Author information

Authors and Affiliations

Authors

Contributions

R.R.III performed the TDTS and the corresponding data analysis. H.T.Y. and S.O. grew the thin films and performed the transport measurements. R.R.III and N.P.A. wrote the manuscript with input from all authors. N.P.A. initiated and supervised the project.

Corresponding authors

Correspondence to Ralph Romero III or N. P. Armitage.

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Extended data

Extended Data Fig. 1 DC resistivity from transport.

ρd.c. of both samples fit with the functional form derived in the main text. The top row shows the full temperature range while the bottom is zoomed in to 50 K. (a), (b) correspond to the x = 0.45 sample and (c), (d) to the x = 0.35 sample.

Extended Data Fig. 2 Fits to the THz conductivity of the x = 0.35.

Figure 2 from the main text for the x = 0.35 sample. a,b σ1, σ2 at a tem- perature (38 K) where a single Drude term suffices. c,d, A temperature (26 K) where a constant offset, σ0, must be in- cluded alongside the Drude term. e,f, A temperature, above Tc, (16 K) where the two fluid model must be invoked. g,h, The lowest temperatures where the conductivity becomes mainly sensitive to the condensate at ν = 0.

Extended Data Fig. 3 Hint of parallel conduction channels.

Experimental motivation for the starting point to derive functional form which fits d.c. data. (a) corresponds to the x = 0.45 sample and b) to the x = 0.35 sample. Error bars represent the 95% confidence interval (2 standard deviations) in the least squares fitting procedure. When not visible they are within the symbol.

Extended Data Fig. 4 Comparison of the optical conductivity of thin films to single crystals.

Comparison of the real part of the optical conductivity of the x = 0.45 thin film (solid lines) in this study and a x = 0.45 single crystal (dashed) measured with FTIR by C. Homes et al, reproduced from (17, 20) At temperatures above the transition (20 and 10 K) the frequency dependence and magnitude are remarkably similar. Below the transition the single crystals appear to show a stronger gap, however these frequencies are at the limit of the FTIR spectrometer. Overall, the qualitative agreement of the spectra give us confidence that we are in the bulk limit.

Extended Data Fig. 5 Lower bound of σ0 for the x = 0.45 sample.

Top row: Here we determine the σ0 which fits the 1 K data, σ0 = 1.0 ± 0.1 mΩ−1cm−1. Fig. 2 (a)–(h), Fig. 3 (a) and (b), Fig. 4 (b), and Extended Data Fig. 3 (a) from the main text with fixed σ0 = 1.0 ± 0.1 mΩ−1cm−1.

Extended Data Fig. 6 Upper bound of σ0 for the x = 0.45 sample.

Here we determine the upper bound of σ0 as when the fits visually do poorly, σ0 = 1.4 ± 0.1 mΩ−1cm−1. Figure 2 (a)–(h), Fig. 3 (a) and (b), Fig. 4 (b), and Extended Data Fig. 3 (a) from the main text with fixed σ0 = 1.4 ± 0.1 mΩ−1cm−1.

Extended Data Fig. 7 Lower bound of σ0 for the x = 0.35 sample.

Top row: Here we determine the σ0 which fits the 1 K data, σ0 = 1.7 ± 0.1 mΩ−1cm−1. Extended Data Fig. 2 (a-h), Fig. 3 (c) and (d), Fig. 4 (d), and Extended Data Fig. 3 (b) from the main text with fixed σ0 = 1.7 ± 0.1 mΩ−1cm−1.

Extended Data Fig. 8 Upper bound of σ0 for the x = 0.35 sample.

Here we determine the upper bound of σ0 as when the fits visually do poorly, σ0 = 2.1 ± 0.1 mΩ−1cm−1. Extended Data Fig. 2 (a)–(h), Fig. 3 (c) and (d), Fig. 4 (d), and Extended Data Fig. 3 (b) from the main text with fixed σ0 = 2.1 ± 0.1 mΩ−1cm−1.

Extended Data Fig. 9 Equivalence of ϵ to two Lorentzians from (20) in low frequency limit.

(a), (b) are Fig. 2 (e), (f) from main text. (c), (d) σ1,2 at 16 K being fit with 2 Drude + 2 Lorentzian model from (20) with the Lorentzians centered at 51 THz (low freq) and 120 THz (high freq). The equivalence of the two methods can be quantified by comparing the fit parameters of the two models. For our model (at 16 K) the narrow Drude has a scattering rate and spectral weight of Γ ≈ 1.2 THz and S ≈ 1.9 mΩ−1cm−1 THz where as the broad Drude (σ0) has a scattering rate and spectral weight orders of magnitude higher than the narrow Drude which we quantified by its DC intercept of σ0 ≈ 1 mΩ−1cm−1. The fit parameters from the two Lorentzian fit are qualitatively equivalent. The narrow Drude from the Lorentzian fit is parameterized by ΓNarrow ≈ 0.9 THz and SNarrow ≈ 1.5 mΩ−1cm−1THz. While the broad Drude from the two Lorentzian fit is parameterized by a DC intercept of σ0 ≈ 1.2 mΩ−1cm−1.

Source data

Source Data Fig. 1 (download XLSX )

Real and imaginary parts of the conductivity as a function of frequency for all measured temperatures.

Source Data Fig. 2 (download XLSX )

Conductivities and relevant fits for the x = 0.45 sample.

Source Data Fig. 3 (download XLSX )

Parameters extracted from the fits in Fig. 2, the linear fits to scattering rates and d.c. resistivities.

Source Data Fig. 4 (download XLSX )

σ2ν and corresponding fits as well as the three measures of superfluid densities.

Source Data Extended Data Fig. 1 (download XLSX )

d.c. resistivities and fit using our derived functional form.

Source Data Extended Data Fig. 2 (download XLSX )

Conductivities and relevant fits for the x = 0.35 sample.

Source Data Extended Data Fig. 3 (download XLSX )

S/Γ, σ0 and 1/ρd.c. values.

Source Data Extended Data Fig. 4 (download XLSX )

Real part of the conductivity for 6, 10 and 20 K (same quantities from refs. 17,20).

Source Data Extended Data Fig. 5 (download XLSX )

Data necessary to reproduce all plots in Extended Data Fig. 5.

Source Data Extended Data Fig. 6 (download XLSX )

Data necessary to reproduce all plots in Extended Data Fig. 6.

Source Data Extended Data Fig. 7 (download XLSX )

Data necessary to reproduce all plots in Extended Data Fig. 7.

Source Data Extended Data Fig. 8 (download XLSX )

Data necessary to reproduce all plots in Extended Data Fig. 8.

Source Data Extended Data Fig. 9 (download XLSX )

Fits to the real and imaginary parts of the conductivity using the two Lorentzian models from ref. 20.

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Romero III, R., Yi, H.T., Oh, S. et al. Planckian scattering and parallel conduction channels in an iron chalcogenide superconductor. Nat. Phys. (2026). https://doi.org/10.1038/s41567-026-03266-8

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